It was indeed used in the 80's polo, but from what I gather it was used since the 1920's.
I should have said up to the 1980's and I have now searched more on the net.
South Crofty sold calcined arsenic (soot) as a bi-product until 1950 when the calciner was no longer used, the residue from the process, mainly iron was stored in the quarry. Changes in processing meant that sulphide tailings was then stored in the quarry for later sale. In the 1970/80's prices were high enough for this to happen and I'm aware that all of the material stored in the quarry was removed during the 1980's.
Other commodity prices crashed with the 1985 tin price crash so sulphide tails were again stored in the quarry until 1988. This has since been buried by mostly inert material.
Baseresult's 2004 GI report for the ROMPs confirms slightly elevated levels towards the bottom of the quarry. The new road's GI report confirms that the highest arsenic level in the entire length of the road was found in material close to the top of the quarry at 1.18%. This is unlikely to be related to processing tails.